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Adrian et al. 1991
Adrian, G.P., Blumenstock, T., Fischer, H., Gerhardt, L., Gulde, T., Oelhaf, H., Thomas, P. and Trieschmann, O. (1991). Column amounts of trace gases derived from ground-based measurements with MIPAS during CHEOPS III. Geophysical Research Letters 18: doi: 10.1029/91GL00551. issn: 0094-8276.

Infrared solar absorption spectra of the atmosphere were taken during the CHEOPS III campaign in Esrange, Sweden in January and February 1990. The MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) instrument used has an unapodized spectral resolution of 0.015 cm-1. Spectra were analysed by means of the SCAIS (Simulation Code for Atmospheric Infrared Spectra) level-by-level and line-by-line algorithm for radiative transfer through the atmosphere. The time series of the retrieved zenith column amounts of O3, H2O, CH4, N2O, HNO3, NO2, HCl, and HF are presented. The stratospheric HCl/HF ratio of 1.3 at the beginning of February, 1990 points towards the conversion of a considerable portion of gaseous HCl to other chemical or physical forms in the stratosphere in this period. A significant change in the HCl column amount between February 4, 1990 and February 8, 1990 was found; this can be correlated with a stratospheric warming between these two dates. From January 27, 1990 to February 11, 1990 the derived upper limits of NO2 abundances were low (≤1.2¿1015 molecules/cm2), whereas the column amounts of HNO3 were very high with 2.9¿1016 molecules/cm2.

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Abstract

Keywords
Atmospheric Composition and Structure, Middle atmosphere—composition and chemistry, Atmospheric Composition and Structure, Transmission and scattering of radiation, Atmospheric Composition and Structure, Instruments and techniques, Meteorology and Atmospheric Dynamics, Polar meteorology
Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
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