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Detailed Reference Information |
Levchenko, V.A., Francey, R.J., Etheridge, D.M., Tuniz, C., Head, J., Morgan, V.I., Lawson, E. and Jacobsen, G. (1996). The 14C “bomb spike” determines the age spread and age of CO2 in Law Dome firn and ice. Geophysical Research Letters 23: doi: 10.1029/96GL03156. issn: 0094-8276. |
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We report a precise, model-independent determination of the age and age spread of CO2 in air trapped in ice. A large pulse of atmospheric radiocarbon, generated in the atmosphere by nuclear tests, peaked in the early-to-mid 1960's. We measure the profile of the radiocarbon ''bomb spike'' in firm air and ice bubbles from high snow-accumulation sites drilled in 1987 and 1993 on Law Dome, East Antarctica, by employing high precision AMS (Accelerator Mass Spectrometry). Large 14C atmospheric growth rates and a high signal-to-noise ratio lead to a direct and precise determination of the CO2 age and age-spread in the ice. A least-squares comparison with the atmospheric history gives a mean CO2 age of 8.9¿0.5 years at the bottom of the firn (where vertical gas diffusion ceases) with an age spread in the ice (full width of a moving average smoothing window) of 12.5¿1.5 years. These results confirm the possibility of examining decadal trace gas variations prior to direct instrumental measurements. |
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Abstract |
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Keywords
Atmospheric Composition and Structure, General or miscellaneous |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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