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Yvon & Butler 1996
Yvon, S.A. and Butler, J.H. (1996). An improved estimate of the oceanic lifetime of atmospheric CH3Br. Geophysical Research Letters 23: doi: 10.1029/95GL03022. issn: 0094-8276.

Previous estimates of the partial atmospheric lifetime of CH3Br with respect to degradation in the ocean have not fully accounted for co-variation of sea-surface and boundary layer properties. Here we substantially reduce uncertainty in this calculation by using a coupled, ocean-atmosphere box model and a tightly gridded data set of oceanic and atmospheric properties. The best estimate of the partial atmospheric lifetime of CH3Br with respect to the ocean is 2.7 y with a possible range, due mainly to the choice of computational procedures for critical terms, of 2.4 to 6.5 y. This range is about one-third of that estimated previously. The total atmospheric lifetime, based upon oceanic, atmospheric, and proposed soil losses with all of their uncertainties, is 0.8 (0.6 to 1.4) y. Only 28% of this total uncertainty is attributable to the uncertainty in oceanic loss. ¿ American Geophysical Union 1996

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Abstract

Keywords
Atmospheric Composition and Structure, Constituent sources and sinks, Atmospheric Composition and Structure, Air/sea constituent fluxes (3339, 4504), Atmospheric Composition and Structure, Troposphere—composition and chemistry
Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
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