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Detailed Reference Information |
McInnes, L., Bergin, M., Ogren, J. and Schwartz, S. (1998). Apportionment of light scattering and hygroscopic growth to aerosol composition. Geophysical Research Letters 25: doi: 10.1029/98GL00127. issn: 0094-8276. |
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During a recent campaign at the NOAA CMDL monitoring station on Sable Island, Canada (43.93 ¿N, 60.01 ¿W) a dual-nephelometer humidigraph measured the hygroscopic growth factor of aerosol scattering, fRB(&sgr;sp), one of the key parameters necessary for estimating short-wave aerosol radiative forcing. Measurements revealed less growth for anthropogenically influenced aerosols than for marine, fRB(&sgr;sp) of 1.7¿0.1 vs. 2.7¿0.4, where fRH(&sgr;sp)=&sgr;sp(85%)/&sgr;sp(40%). A combined measurement-modeling approach was used to estimate &sgr;sp and its RH-dependence, based on the measured particle size distribution and composition. The model suggested that differences in the particle size distribution, assuming the same aerosol composition, could not explain the observed differences in fRH(&sgr;sp). We have confirmed with individual particle analysis, that aerosol composition was indeed responsible for the difference in fRH(&sgr;sp). As well, the scattering contribution of organic carbon for the influenced case is at least as much as sulfate aerosol. ¿ 1998 American Geophysical Union |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Pollution—urban and regional, Atmospheric Composition and Structure, Transmission and scattering of radiation, Atmospheric Composition and Structure, Instruments and techniques |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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