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Harnisch et al. 1998
Harnisch, J., Bischof, W., Borchers, R., Fabian, P. and Maiss, M. (1998). A stratospheric excess of CO2-due to tropical deep convection?. Geophysical Research Letters 25: doi: 10.1029/97GL03398. issn: 0094-8276.

The 'age' of stratospheric air is a measure that characterizes the time scales of stratospheric transport. In this work we present and compare age-values as determined from measurements of CO2 and SF6 on air-samples obtained between 1987 and 1995 on six flights of our balloon-borne cryo-sampler. In the middle stratosphere for five out of six flights we find age-values that are up to three years lower for CO2 than for SF6. This CO2-age anomaly corresponds to an excess of 4--5 ppm CO2. Evidence is presented that this excess-CO2 originates from rapid convective transport of near surface air. Additionally, we show that globally no compact relationship exists between the age of air and mixing-ratios of N2O. ¿ 1998 American Geophysical Union

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Abstract

Keywords
Atmospheric Composition and Structure, Middle atmosphere—composition and chemistry, Atmospheric Composition and Structure, Troposphere—composition and chemistry, Meteorology and Atmospheric Dynamics, Convective processes, Meteorology and Atmospheric Dynamics, General circulation
Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
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