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Weisenstein et al. 1997
Weisenstein, D.K., Yue, G.K., Ko, M.K.W., Sze, N., Rodriguez, J.M. and Scott, C.J. (1997). A two-dimensional model of sulfur species and aerosols. Journal of Geophysical Research 102: doi: 10.1029/97JD00901. issn: 0148-0227.

A two-dimensional model of sulfate aerosols has been developed. The model includes the sulfate precursor species H2S, CS2, DMS, OCS, and SO2. Microphysical processes simulated are homogeneous nucleation, condensation and evaporation, coagulation, and sedimentation. Tropospheric aerosols are removed by washout processes and by surface deposition. We assume that all aerosols are strictly binary water-sulfuric acid solutions without solid cores. The main source of condensation nuclei for the stratosphere is new particle formation by homogeneous nucleation in the upper tropical troposphere. A significant finding is that the stratospheric aerosol mass may be strongly influenced by deep convection in the troposphere. This process, which could transport gas-phase sulfate precursors into the upper troposphere and lead to elevated levels of SO2 there, could potentially double the stratospheric aerosol mass relative to that due to OCS photooxidation alone. Our model is successful at reproducing the magnitude of stratospheric aerosol loading following the Mount Pinatubo eruption, but the calculated rate of decay of aerosols from the stratosphere is faster than that derived from observations.¿ 1997 American Geophysical Union

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Abstract

Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Middle atmosphere—composition and chemistry, Atmospheric Composition and Structure, Volcanic effects, Atmospheric Composition and Structure
Journal
Journal of Geophysical Research
http://www.agu.org/journals/jb/
Publisher
American Geophysical Union
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