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Detailed Reference Information |
Glatthor, N., Blom, C.E., von Clarmann, T., Fischer, H., Gulde, T., Piesch, C., Erle, F., Pfeilsticker, K., Chipperfield, M.P., Lee, A.M. and Pyle, J.A. (1998). Airborne remote sensing of NO2 in the Arctic winter of 1994–1995 and comparison with a three-dimensional chemical transport model. Journal of Geophysical Research 103: doi: 10.1029/98JD00521. issn: 0148-0227. |
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In the winter of 1994--1995, for the first time NO2 was observed by the Michelson Interferometer for Passive Atmospheric Sounding-Flugzeug Transall (MIPAS-FT). We present the NO2 data of MIPAS and of a Differential Optical Absorption Spectroscopy (DOAS) instrument, which was also operated on the Transall, and compare the measurements with the Single Layer Isentropic Model for Chemistry And Transport (SLIMCAT). The daytime midlatitude NO2 column amounts of MIPAS and DOAS increased from 1¿1015 cm-2 in December to ~3¿1015 cm-2 in March. After sunset MIPAS observed strong NO2 increases, up to 3.2¿1015 cm-2 on December 20, up to 7.2¿1015 cm-2 on January 17 and up to 6.4¿1015 cm-2 on March 27. These high nighttime values, showing considerable amounts of NOx in the midlatitude stratosphere, were qualitatively reproduced by SLIMCAT. The NO2 columns measured inside the Arctic vortex, ≤1¿1015 cm-2 from December until mid-January with no substantial increase after sunset, displayed strong denoxification. From the end of January the Arctic daytime NO2 columns grew to ~2¿1015 cm-2, and after sunset MIPAS observed similar strong increases as at midlatitudes, up to 3.4¿1015 cm-2 on January 24 and up to 4.8¿1015 cm-2 in March and April. The renoxification of the vortex was also shown by SLIMCAT. On April 5, MIPAS NO2 column amounts decreased by 1.5¿1015 cm-2 after reaching the maximum, caused by N2O5 and ClONO2 formation and encounter of less renoxified air masses. ¿ 1998 American Geophysical Union |
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BACKGROUND DATA FILES |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Constituent sources and sinks, Atmospheric Composition and Structure, Middle atmosphere—composition and chemistry, Atmospheric Composition and Structure, Middle atmosphere—constituent transport and chemistry, Atmospheric Composition and Structure, Instruments and techniques |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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