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Detailed Reference Information |
Kulmala, M., Toivonen, A., Mattila, T. and Korhonen, P. (1998). Variations of cloud droplet concentrations and the optical properties of clouds due to changing hygroscopicity: A model study. Journal of Geophysical Research 103: doi: 10.1029/98JD00880. issn: 0148-0227. |
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The effects of the availability of gaseous nitric acid, hydrochloric acid, and ammonia on cloud droplet formation have been studied using an adiabatic air parcel model including detailed multicomponent condensation. The used preexisting lognormal particle distribution is bimodal in size and in hygroscopicity: four lognormal distributions were used. In each mode particles were assumed to be internally mixed; that is, they were composed partly of salt and partly of an insoluble substance. According to the simulations made, a clear positive correlation between condensable species concentrations and the number of activated cloud droplets exists. Thus trace gases can also influence the optical thickness and reflectance of clouds. The simulations show that ammonia enhances the condensation rate of acids and thus also their effect on the cloud droplet activation significantly. The change in optical thickness varies as a function of the number concentration of preexisting particles, having a maximum (Δ&tgr;/&tgr;=1.6) near a concentration of 1000--2000 cm-3. ¿ 1998 American Geophysical Union |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Cloud physics and chemistry, Atmospheric Composition and Structure, Transmission and scattering of radiation, Atmospheric Composition and Structure, Troposphere—composition and chemistry |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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