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Hurst et al. 1998
Hurst, D.F., Bakwin, P.S. and Elkins, J.W. (1998). Recent trends in the variability of halogenated trace gases over the United States. Journal of Geophysical Research 103: doi: 10.1029/98JD01879. issn: 0148-0227.

Recent trends in the atmospheric variability of seven halogenated trace gases are determined from three years (November 1994 through October 1997) of hourly gas chromatographic measurements at a 610 m tower in North Carolina and 17 months (June 1996 through October 1997) of similar measurements at a 450 m tower in Wisconsin. Production of five of these gases, CCl3F (CFC-11), CCl2F2 (CFC-12), CCl2FCClF2 (CFC-113), CH3CCl3 (methyl chloroform), and CCl4 (carbon tetrachloride), is now strictly regulated in the United States and other developed countries under international legislation. C2Cl4 (tetrachloroethene) and SF6 (sulfur hexafluoride) are currently produced without restriction, but requests for voluntary cutbacks in C2Cl4 emissions have been made, at least in the United States. Atmospheric variability of these gases is examined at several sampling heights on the towers, but trends are deduced using only nighttime data at the top sampling level of each tower to minimize variability driven by local emissions and the diurnal cycle of the planetary boundary layer, leaving regional emissions as the main source of day-to-day variability. Significant downward trends are determined for CFC-12, CFC-113, CH3CCl3, and C2Cl4 variability at both towers, reflecting decreased emissions of these gases in two regions of the United States. Trends in CFC-11, CCl4, and SF6 variability at both towers are not significantly different from zero. ¿ 1998 American Geophysical Union

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Keywords
Atmospheric Composition and Structure, Constituent sources and sinks, Atmospheric Composition and Structure, Pollution—urban and regional, Atmospheric Composition and Structure, Troposphere—composition and chemistry, Meteorology and Atmospheric Dynamics, Boundary layer processes
Journal
Journal of Geophysical Research
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Publisher
American Geophysical Union
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