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Choi et al. 2001
Choi, J.C., Lee, M., Chun, Y., Kim, J. and Oh, S. (2001). Chemical composition and source signature of spring aerosol in Seoul, Korea. Journal of Geophysical Research 106: doi: 10.1029/2001JD900090. issn: 0148-0227.

The measurement of atmospheric aerosol was made in Seoul during the spring of 1998. The objective of this study was to investigate the chemical characteristics of atmospheric aerosol with an emphasis on the effect of Asian dust. Total suspended particles (TSP) and particles smaller than 10 μm (PM10) were collected during March--May 1998. For PM10, water-soluble ions and trace elements were analyzed: NO3-, SO42-, Na+, NH4+, K+, Mg2+, Ca2+, Na, Mg, Al, Ca, Fe, Mn, Cr, Co, Cu, Zn, Cd, and Pb. All data were sorted into three groups on the basis of the intensity of Asian dust observed in Seoul: nondust, regular dust, and heavy dust. Chemical characteristics of aerosol were distinct for the heavy dust incidence compared to the other two cases. The average mass concentration of TSP and PM10 increased substantially during the heavy dust period. For water-soluble ions, concentrations of SO42- and NO3- were the lowest, whereas Ca2+ and Mg2+ concentrations were remarkably enhanced. Concentrations and mass fraction of crustal elements such as Na, Mg, Ca, Fe, and Mn were highly elevated, but those of pollution-derived heavy metals were appreciably decreased. Enrichment ratios of metallic components indicated that soil dust was the primary source of spring aerosols over Seoul. This was also confirmed by factor analysis. Trajectory analysis provided a convincing evidence for the air mass coming from the Asian desert areas, which are the source region of mineral dust. In contrast, the anthropogenic influence was more pronounced for the regular dust period: concentrations of heavy metals, NO3-, and SO42- were the highest. It could be associated with the transport of air mass over the industrialized regions of China, which is demonstrated by backward trajectory analysis. The result of factor analysis with high factor loadings in SO42- and NO3- implied the considerable influence of industrial emission on the composition of all spring aerosols over Korea. ¿ 2001 American Geophysical Union

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Abstract

Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Constituent sources and sinks, Atmospheric Composition and Structure, Troposphere—composition and chemistry, Atmospheric Composition and Structure, Troposphere—constituent transport and chemistry
Journal
Journal of Geophysical Research
http://www.agu.org/journals/jb/
Publisher
American Geophysical Union
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