Meteorological highlights from the third NASA Global Tropospheric Experiment Chemical Instrumentation Test and Evaluation (GTE/CITE 3) are presented. During August and September 1989, research flights were conducted from Wallops Island, Virginia, and Natal, Brazil, and included airborne sampling of air masses over adjacent regions of the Atlantic Ocean. Isentropic backward trajectory calculations, wind vector/streamline fields, rawinsonde data, and GOES and METEOSAT satellite imagery are utilized to examine the meteorological conditions for each flight and to determine the transport paths of the sampled air masses. Some aspects of the chemical signatures of the sampled air are also discussed. During the series of flights based at Wallops Island, Virginia, the flow into the experiment area was governed primarily by the position of the North Atlantic subtropical anticyclone. The large-scale tropospheric circulation switched from primarily a marine flow during flights 1--4, to a predominantly offshore mid-latitude continental flow during flights 5--10. During these later flights, the regional influences of large eastern U. S. cities along with vertical mixing by typical summertime convective activity strongly influenced the chemical characteristics of the sampled air. During the series of flights based at Natal, Brazil, the dominant synoptic feature was the South Atlantic subtropical anticyclone which generally transported air across the tropical Atlantic toward eastern Brazil. Pronounced subsidence and a well-defined trade wind inversion often characterized the lower and middle troposphere over the Natal region. Some high-altitude recirculation of air from South America was observed, as was cross-equatorial transport which had come from northern Africa. Biomass burning plumes were observed on segments of all of the flights, the source region being the central and southern savannah regions of Africa. ¿ American Geophysical Union 1993