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Detailed Reference Information |
Tilmes, S., Müller, R., Grooß, J., Höpfner, M., Toon, G.C. and Russell, J.M. (2003). Very early chlorine activation and ozone loss in the Arctic winter 2002–2003. Geophysical Research Letters 30: doi: 10.1029/2003GL018079. issn: 0094-8276. |
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Chlorine activation and chemical ozone destruction is investigated in the Arctic winter 2002--03 using the tracer-tracer correlation technique. Consistent with very low temperatures in the early vortex, strong chlorine activation at 520 K potential temperature was observed already in mid-December 2002 by the MkIV balloon and at 400--500 K in early January 2003 from HALOE satellite measurements. Large column ozone loss was derived inside the outer vortex in January (23 ¿ 9 DU) and substantially greater losses in February (51 ¿ 9 DU) inside the vortex core in 380--550 K. Calculated ozone loss is similar in February in the two completely separated parts of the vortex. Little influence of mixing in of mid-latitude is noticeable after the reunification of the vortex. Further, some ozone loss at lower altitudes likely occurred during March and April consistent with polar stratospheric clouds detected by MIPAS-ENVISAT towards the end of March. |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Middle atmosphere--composition and chemistry, Atmospheric Composition and Structure, Middle atmosphere--constituent transport and chemistry, Atmospheric Composition and Structure, Instruments and techniques |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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