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Detailed Reference Information |
Irie, H., Kondo, Y., Koike, M., Takegawa, N., Tabazadeh, A., Reeves, J.M., Sachse, G.W., Vay, S.A., Anderson, B.E. and Mahoney, M.J. (2004). Liquid ternary aerosols of HNO3/H2SO4/H2O in the Arctic tropopause region. Geophysical Research Letters 31: doi: 10.1029/2003GL018678. issn: 0094-8276. |
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Measurements of total reactive nitrogen (NOy) concentrations in the gas and aerosol phases were made on board the NASA DC-8 aircraft within 1 km above the Arctic tropopause in February 2000. As temperatures decreased, NOy was taken up into the background sulfate aerosols. The observed temperature-dependent NOy uptake agrees well with that calculated from a model of nitric acid (HNO3) uptake to form liquid HNO3/H2O/H2SO4 ternary droplets. The observations reported here provide the first direct evidence for the formation of ternary droplets in the Arctic tropopause region. |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Aerosols and particles, Atmospheric Composition and Structure, Cloud physics and chemistry, Atmospheric Composition and Structure, Middle atmosphere—composition and chemistry |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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