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Thompson et al. 2003
Thompson, A.M., Witte, J.C., Oltmans, S.J., Schmidlin, F.J., Logan, J.A., Fujiwara, M., Kirchhoff, V.W.J.H., Posny, F., Coetzee, G.J.R., Hoegger, B., Kawakami, S., Ogawa, T., Fortuin, J.P.F. and Kelder, H.M. (2003). Southern Hemisphere Additional Ozonesondes (SHADOZ) 1998–2000 tropical ozone climatology 2. Tropospheric variability and the zonal wave-one. Journal of Geophysical Research 108: doi: 10.1029/2002JD002241. issn: 0148-0227.

The first view of stratospheric and tropospheric ozone variability in the Southern Hemisphere tropics is provided by a 3-year record of ozone soundings from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network (http://croc.gsfc.nasa.gov/shadoz). Observations covering 1998--2000 were made over Ascension Island, Nairobi (Kenya), Irene (South Africa), R¿union Island, Watukosek (Java), Fiji, Tahiti, American Samoa, San Crist¿bal (Galapagos), and Natal (Brazil). Total, stratospheric, and tropospheric column ozone amounts usually peak between August and November. Other features are a persistent zonal wave-one pattern in total column ozone and signatures of the quasi-biennial oscillation (QBO) in stratospheric ozone. The wave-one is due to a greater concentration of free tropospheric ozone over the tropical Atlantic than the Pacific and appears to be associated with tropical general circulation and seasonal pollution from biomass burning. Tropospheric ozone over the Indian and Pacific Oceans displays influences of the waning 1997--1998 El Ni¿o, seasonal convection, and pollution transport from Africa. The most distinctive feature of SHADOZ tropospheric ozone is variability in the data, e.g., a factor of 3 in column amount at 8 of 10 stations. Seasonal and monthly means may not be robust quantities because statistics are frequently not Gaussian even at sites that are always in tropical air. Models and satellite retrievals should be evaluated on their capability for reproducing tropospheric variability and fine structure. A 1999--2000 ozone record from Paramaribo, Surinam (6¿N, 55¿W) (also in SHADOZ) shows a marked contrast to southern tropical ozone because Surinam is often north of the Intertropical Convergence Zone (ITCZ). A more representative tropospheric ozone climatology for models and satellite retrievals requires additional Northern Hemisphere tropical data.

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Abstract

Keywords
Atmospheric Composition and Structure, Troposphere--composition and chemistry, Global Change, Remote sensing, Meteorology and Atmospheric Dynamics, Climatology, Information Related to Geographic Region, Africa, Information Related to Geographic Region, Atlantic Ocean
Journal
Journal of Geophysical Research
http://www.agu.org/journals/jb/
Publisher
American Geophysical Union
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