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Detailed Reference Information |
Klaminder, J., Renberg, I., Bindler, R. and Emteryd, O. (2003). Isotopic trends and background fluxes of atmospheric lead in northern Europe: Analyses of three ombrotrophic bogs from south Sweden. Global Biogeochemical Cycles 17. doi: 10.1029/2002GB001921. issn: 0886-6236. |
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Knowledge about the natural atmospheric background deposition rate of lead (Pb) prior to anthropogenic pollution is critical in the understanding of present-day pollution and for establishing realistic goals for the reduction of atmospheric Pb. We utilize stable Pb isotopes (206Pb and 207Pb) in radiocarbon-dated peat cores from three ombrotrophic bogs from south Sweden, to calculate fluxes and to survey atmospheric Pb trends prior 3500 BP (the so far known onset of large-scale anthropogenic pollution). The estimated atmospheric Pb deposition rate was between 1 and 10 ¿g Pb m2 yr-1 between 5900 and 3700 calendar years BP, which is 100 to 1000 times lower than present-day deposition rates. The majority of the samples older than 3500 calendar years BP had 206Pb/207Pb ratios ≤1.20, which is significantly lower than unpolluted Swedish mineral soils (206Pb/207Pb > 1.30), suggesting that even the natural atmospheric deposition of Pb was dominated by long-range transport, rather than local inputs from soil dust. Low 206Pb/207Pb ratios (1.16--1.18) of several samples indicate that this distant transport originated at least partly from early pollution sources. A possible climatic connection with the observed Pb deposition trends is suggested. |
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Abstract |
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Keywords
Atmospheric Composition and Structure, Pollution--urban and regional, Geochemistry, Isotopic composition/chemistry, Geochemistry, Trace elements, Information Related to Geographic Region, Europe |
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Publisher
American Geophysical Union 2000 Florida Avenue N.W. Washington, D.C. 20009-1277 USA 1-202-462-6900 1-202-328-0566 service@agu.org |
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