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Harvey 2003
Harvey, L.D.D. (2003). Impact of deep-ocean carbon sequestration on atmospheric CO2 and on surface-water chemistry. Geophysical Research Letters 30: doi: 10.1029/2002GL016224. issn: 0094-8276.

The effectiveness of injection into the ocean of CO2 produced from the use of fossil fuels is investigated using a coupled climate-carbon cycle model. Four fossil fuel emission scenarios are considered, in which emissions peak at 28 Gt C/yr in 2100 (scenario 1), 9 Gt C/yr in 2050 (scenario 2), or decrease to zero by 2100 or 2075 (scenarios 3 and 4). Sequestration sufficient to reduce the net emissions for scenarios 1--3 to that in scenario 4 is considered. Sequestration in scenario 1 results in a CO2 concentration of 857 ppmv by 3100, compared to a peak of 1614 ppmv without sequestration, and slows the accumulation of atmospheric CO2. The supersaturation of the non-polar mixed layer with respect to calcite decreases from 486% pre-industrial to about 250%, while mixed layer pH decreases by 0.66. Only for scenario 3 is sequestration sufficient to limit the peak impact on atmospheric CO2 and mixed layer chemistry to the impacts obtained in scenario 4.

BACKGROUND DATA FILES

Abstract

Keywords
Oceanography, Biological and Chemical, Carbon cycling, Global Change, Biogeochemical processes, Global Change, Climate dynamics, Global Change, Oceans
Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
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