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Lamarque et al. 2002
Lamarque, J.-F., Khattatov, B.V. and Gille, J.C. (2002). Constraining tropospheric ozone column through data assimilation. Journal of Geophysical Research 107: doi: 10.1029/2001JD001249. issn: 0148-0227.

Global distributions of the tropospheric ozone column (TOC) and its error are estimated by assimilating satellite observations of total ozone column and stratospheric ozone profiles in a global chemistry-transport model. A quantitative comparison of the calculated TOC with collocated ozonesondes observations shows good agreement over a wide range of latitudes for the period studied (July--September 1992), even at the daily timescale. In most cases, the difference with the ozonesonde-based TOC is within the calculated error estimate. Comparison with the TOC distribution by Thompson and Hudson <1999> does not lead to any quantitative conclusion due to a mix of similarities and differences, even in the geographical distribution of the TOC. A positive TOC bias with respect to ozonesondes is found in this study over Hilo and Irene, probably due to a misrepresentation of the transport of ozone in a region of strong TOC gradients. In September 1992 the LIDAR observations from the TRACE-A campaign are also assimilated. This is shown to provide a constraint on the TOC that significantly propagates across the Atlantic Ocean, indicating the importance of point measurements of ozone for constraining its large-scale distribution.

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Abstract

Keywords
Atmospheric Composition and Structure, Pollution--urban and regional, Atmospheric Composition and Structure, Troposphere--composition and chemistry, Meteorology and Atmospheric Dynamics, Numerical modeling and data assimilation
Journal
Journal of Geophysical Research
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Publisher
American Geophysical Union
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