EarthRef.org Reference Database (ERR)
Development and Maintenance by the EarthRef.org Database Team

Detailed Reference Information
Meskhidze et al. 2003
Meskhidze, N., Chameides, W.L., Nenes, A. and Chen, G. (2003). Iron mobilization in mineral dust: Can anthropogenic SO2 emissions affect ocean productivity?. Geophysical Research Letters 30: doi: 10.1029/2003GL018035. issn: 0094-8276.

For Fe contained in long-range transported aeolian dust to act as a micronutrient for oceanic phytoplankton it must be first dissolved or mobilized. We propose that Fe-mobilization can occur in mineral dust from East Asia by the incorporation of SO2 into the advecting dust plumes and subsequent acidification of the dust through heterogeneous SO2 oxidation. To test this hypothesis, we consider a dust plume that originated from the gobi-deserts and advected over the Pacific Ocean. Data collected over the Yellow Sea confirm that this plume contained high concentrations of dust and SO2. Significant gaseous HNO3 concentrations indicate that the dust particles were acidified (i.e., pH < 2). At these pH's, 1--2% of the Fe contained in a deliquescent mineral dust particle would be mobilized within 3--5 days. These results suggest a possible link between the rate of C-fixation in so-called High-Nitrate-Low-Chlorophyll regions of the Pacific Ocean and SO2 emissions from East Asia.

BACKGROUND DATA FILES

Abstract

Keywords
Atmospheric Composition and Structure, Air/sea constituent fluxes (3339, 4504), Atmospheric Composition and Structure, Geochemical cycles, Atmospheric Composition and Structure, Pollution--urban and regional, Oceanography, Biological and Chemical, Aerosols, Oceanography, Biological and Chemical, Trace elements
Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
2000 Florida Avenue N.W.
Washington, D.C. 20009-1277
USA
1-202-462-6900
1-202-328-0566
service@agu.org
Click to clear formClick to return to previous pageClick to submit