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Sekiguchi et al. 2003
Sekiguchi, M., Nakajima, T., Suzuki, K., Kawamoto, K., Higurashi, A., Rosenfeld, D., Sano, I. and Mukai, S. (2003). A study of the direct and indirect effects of aerosols using global satellite data sets of aerosol and cloud parameters. Journal of Geophysical Research 108: doi: 10.1029/2002JD003359. issn: 0148-0227.

The present study investigated the correlations between aerosol and cloud parameters derived from satellite remote sensing for evaluating the radiative forcing of the aerosol indirect effect. The global statistics showed that the effective particle radius and the optical thickness of low clouds correlate well with the column number concentration of the aerosol particles, indicating an aerosol indirect effect. A correlation of the cloud fraction with the aerosol number was also seen, whereas we could not find a significant correlation of the cloud-top temperature with the column aerosol number. Furthermore, the regional statistics presented that positive correlations between the cloud optical thickness and cloud fraction with the aerosol column number concentration exist in most regions consistent with the global mean statistics. However, the effective cloud particle radius showed a tendency similar to the global correlation only around the seashore regions. Using these correlations and assuming that the aerosol column number concentration has increased by 30% from the preindustrial era, the total radiative forcing of the aerosol indirect effect was evaluated to be about -0.6 to -1.2 W m-2. The radiative forcing of the aerosol direct effect from the satellite-retrieved parameters was also evaluated as -0.4 W m-2 over the ocean. The cloud-top temperature was found to be insensitive to the change in the aerosol number, although there was a distinct negative correlation between the aerosol number and cloud temperature at which the cloud particle grows to a radius of 14 ¿m. This particular dependency of the cloud temperature suggests that aerosols acts on clouds so as to change cloud particle size near the cloud top, optical thickness, and fraction but to keep their cloud-top temperature without causing a significant longwave radiative forcing.

BACKGROUND DATA FILES

Abstract

Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Cloud physics and chemistry, Meteorology and Atmospheric Dynamics, Radiative processes, Meteorology and Atmospheric Dynamics, Remote sensing
Journal
Journal of Geophysical Research
http://www.agu.org/journals/jb/
Publisher
American Geophysical Union
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