EarthRef.org Reference Database (ERR)
Development and Maintenance by the EarthRef.org Database Team

Detailed Reference Information
Rowland et al. 1982
Rowland, F.S., Tyler, S.C., Montague, D.C. and Makide, Y. (1982). Dichlorodifluoromethane, CCl2F2, in the earth’s atmosphere. Geophysical Research Letters 9: doi: 10.1029/GL009i004p00481. issn: 0094-8276.

Atmospheric observations of CCl2F2 concentrations from 1976--1980 (Rasmussen et al., 1981) have been compared with atmospheric models containing stratospheric destruction alone, and with various added hypothetical tropospheric sinks ranging from 10--100 year lifetimes. Comparisons are made using (a) absolute atmospheric burdens of CCl2F2; (b) the time trend of relative concentrations; and (c) the ratio of concentrations measured in the northern and southern hemispheres. The atmospheric emissions of CCl2F2 estimated by the Chemical Manufacturers Association (CMA) fail to fit the observations with stratospheric loss alone in all three tests. The inclusion of tropospheric loss processes appreciably worsens the agreement. Three other hypothetical emissions estimates are given which satisfactorily simulate the atmospheric observations by all three tests. The emissions in these models maximize in 1978 or later at more than 500 kilotons/year, in contrast to the CMA maximum of 420 kilotons during 1974. The total emissions of CCl2F2 during 1976 through 1979 in these other models are about 35% greater than in the CMA estimates.

BACKGROUND DATA FILES

Abstract

Journal
Geophysical Research Letters
http://www.agu.org/journals/gl/
Publisher
American Geophysical Union
2000 Florida Avenue N.W.
Washington, D.C. 20009-1277
USA
1-202-462-6900
1-202-328-0566
service@agu.org
Click to clear formClick to return to previous pageClick to submit