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Hofmann & Rosen 1983
Hofmann, D.J. and Rosen, J.M. (1983). Stratospheric sulfuric acid fraction and mass estimate for the 1982 volcanic eruption of El Chichon. Geophysical Research Letters 10: doi: 10.1029/GL010i004p00313. issn: 0094-8276.

From baloon-borne particle counter data at Laramie (41¿N) and in southern Texas (27-29 ¿N), the total stratospheric mass of the eruptions of El Chichon is estimated to be ≈8 Tg about 6 1/2 months after the eruption with possibly as much as 20 Tg in the stratosphere about 45 days after the eruption. The aerosol as observed in Texas was primarily in two layers, both highly volatile (≥98%) at 150 ¿C. Aerosol in the upper layer at ≈25 km was composed of an ≈80% H2SO4 solution while the lower layer at ≈18 km was composed of a 60-65% H2SO4 solution aerosol. An H2SO4 vapor concentration of at least 3¿107 molecules cm-3 is estimated as needed to sustain the large droplets in the upper layer. An early bi-modal nature in the size distribution suggested droplet nucleation from the gas phase during the first 3 months and similarity of the large particle profiles 2 months apart indicated continued particle growth 6 1/2 months after the eruption. By December, the aerosol layers had largely spread to the latitude of Laramie (41 ¿N).

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Geophysical Research Letters
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American Geophysical Union
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