The magnitude of beam attenuation attributed to suspended sediments, cp, and the slope of the log-transformed attenuation spectrum, γ, were used to investigate the properties and dynamic nature of matter suspended in the waters of western Long Island Sound (LIS) and the adjacent Connecticut River plume (CRP). Within the LIS, cp and γ indicate a robust relationship between sediment concentration and particle size distribution (PSD). As concentration increased, the PSD shifted to larger particles. The highest concentrations and particle sizes were found in a nepheloid layer adjacent to the sound floor. Within the adjacent CRP, sediments were observed to shift towards smaller particles at the lateral plume boundary, where current shear stress may have disrupted large particle aggregates, relative to sediments in the more quiescent plume interior. A strong linear correlation between γ and salinity was also found, indicating that mixing between the two water masses may also have altered the PSD of the plume sediments. A suspended sediment attenuation model based on Mie theory, a power law form of the PSD, and a single sediment source indicates that the observed changes in LIS cp and γ are consistent with sediment removal as particles settle with size-dependent rates. In contrast, within the CRP, the model supports the hypothesis that turbulence-induced aggregate disruption at the lateral plume boundary is responsible for the observed variability in cp and γ. However, mixing between the LIS and CRP particle populations would violate the single source requirement of the model and necessitate a more complicated set of particle dynamics in order to correctly interpret the observed variability in particulate attenuation.