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Brown et al. 1996
Brown, R.C., Miake-Lye, R.C., Anderson, M.R. and Kolb, C.E. (1996). Effect of aircraft exhaust sulfur emissions on near field plume aerosols. Geophysical Research Letters 23: doi: 10.1029/96GL03338. issn: 0094-8276.

A two dimensional, axisymmetric flowfield model with coupled gas phase oxidation kinetics and aerosol nucleation and growth dynamics is used to evaluate the effect of fuel sulfur oxidation in the Concorde engine on the formation and growth of volatile H2SO4/H2O aerosols in the near field plume. Based on estimated exit plane sulfur speciation, results are shown for between 2% and 20% conversion of the fuel sulfur to S(VI) (SO3 and H2SO4) in engine. The primary motivation is to provide estimates for the changes in the number density and surface area density of sulfuric acid aerosols due to sulfur oxidation in the engine. This analysis indicates the need for experimental measurements of sulfur emissions at the exhaust exit, in addition to soot properties, to fully assess the atmospheric impact of aircraft emissions. ¿ American Geophysical Union 1996

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Abstract

Keywords
Meteorology and Atmospheric Dynamics, General or miscellaneous
Journal
Geophysical Research Letters
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Publisher
American Geophysical Union
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