A simple quasi-two-dimensional model is used to study the zonal distribution of NOx. The model includes vertical transport in the form of eddy diffusion and deep convection, zonal transport by a vertical uniform wind, and a simplified chemistry of NO, NO2, and HNO3. The NOx sources considered are surface emissions (mostly from the combustion of fossil fuel), lightning, aircraft emissions, and downward transport from the stratosphere. The model is applied to the latitude band of 40¿ and 50¿N during the month of June; the contributions to the zonal NOx distribution from the individual sources and transport processes are investigated. The model predicted NOx concentration in the upper troposphere is dominated by air lofted from the polluted planetary boundary layer over the large industrial areas of eastern North America and Europe. Aircraft emissions are also important and contribute on average 30%. Stratospheric input is minor about 10%, less even than that by lightning. The model provides a clear indication of intercontinental transport of NOx and HNO3 in the upper troposphere. Comparison of the modeled NO profiles over the western Atlantic with those measured during STRATOZ III in 1984 shows good agreement at all altitudes. ¿ American Geophysical Union 1992 |