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Kleefeld et al. 2002
Kleefeld, C., O'Dowd, C.D., O'Reilly, S., Jennings, S.G., Aalto, P., Becker, E., Kunz, G. and de Leeuw, G. (2002). Relative contribution of submicron and supermicron particles to aerosol light scattering in the marine boundary layer. Journal of Geophysical Research 107: doi: 10.1029/2000JD000262. issn: 0148-0227.

Measurements of the aerosol light scattering coefficient (σsp) at a wavelength of λ = 550 nm were conducted at a coastal atmospheric research station in the east Atlantic Ocean during June 1999. Size distribution measurements between diameters of 3 nm and 40 ¿m (at ambient humidity) were used to derive scattering coefficients from Mie theory. The calculated scattering coefficients were about a factor of 7.4 higher than the measured scattering coefficients. The discrepancy was explained by a reduced cutoff of the sampling system at particle diameters between 6 and 8 ¿m, dependent on wind speed. The calculated aerosol scattering was about 1 order of magnitude higher than previously reported measurements in the MBL and is attributed to supermicrometer particles at sizes d > 10 ¿m dominating aerosol scattering.

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Abstract

Keywords
Atmospheric Composition and Structure, Aerosols and particles (0345, 4801), Atmospheric Composition and Structure, Transmission and scattering of radiation, Meteorology and Atmospheric Dynamics, Radiative processes
Journal
Journal of Geophysical Research
http://www.agu.org/journals/jb/
Publisher
American Geophysical Union
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